Paper 1.1

 

The Complex World of Plutonium Science

 

Massalski Thaddeus B.1  and  Hecker Siegfried S.2

 

1Carnegie Mellon University, Pittsburgh PA, U.S.A

 2 Los Alamos National Laboratory, Los Alamos NM,  U.S.A.

 

Plutonium is a metal of great interest because of its most unusual  metallurgical, electronic, and nuclear properties.  In the Periodic Table,  it sits in the middle of the actinide series, and there it occupies a  unique position, unlike any other element.  It exhibits six solid  allotropic changes, at ordinary pressure, and is strikingly unstable with  temperature, pressure, chemical additions, and time.  It undergoes  virtually every type of phase transformation known.  In the solid state,  the 5f electrons of Pu are caught in an abrupt transition between being  localized and contributing to bonding.  The proximity of the 7s, 6d, and 5f  electrons in the valence orbitals leads to many complex electronic  interactions and physical properties. 

 

The intepretation of many of the  above features is a challenge to both physics and materials science.